You need to create the ufl expression and then project it to some space. I will use the following:
V = FunctionSpace(mesh, 'CG', 1)
Now, use the following:
f = psiinit( element = FiniteElement('CG', mesh.ufl_cell(), 3))
lap = div(grad(f))
lap would be enough to create a form. If you need to plot it or evaluate it, projection would be required:
Plap = project(lap, V)
Note that I used degree = 3 in f, because derivation is done at the discrete level, so less than 2 will give a null laplacian.
Best regards!